Study of 2-(piperidine-1-ylmethyl)cyclohexanamine structure synthesis based on oxime protected compounds in mannich mechanism

Taheri, M; Soleymani, R; Hosn, B; Rajabzadeh, H; Darvish, MR

HERO ID

8721700

Reference Type

Journal Article

Year

2012

Language

English

HERO ID 8721700
In Press No
Year 2012
Title Study of 2-(piperidine-1-ylmethyl)cyclohexanamine structure synthesis based on oxime protected compounds in mannich mechanism
Authors Taheri, M; Soleymani, R; Hosn, B; Rajabzadeh, H; Darvish, MR
Journal Oriental Journal of Chemistry
Volume 28
Issue 1
Page Numbers 387-397
Abstract 2-(piperidine-1 -ylmethyl)cyclohexanone (PMC), 2-(piperidine-1 -ylmethyl)cyclohexanone oxime (PMCO) structures and also 2-(piperidirte-1- ylmethyl) cyclohexan amine (PMCA) structure were extracted using experimental methods of Mannich reaction, based on oxime protected compounds. The given structures were purified at the end of syntheses process, by chromatography column. Related structures were identified by using 13C-NMR, 1H-NMR, FT-IR and mass spectroscopy. Attained results showed that using oxime structure as an intermediate causes to increase the yield and also to increase reaction ratio attain final product. However, all the attained spectra approved existence of intermediate and the final product. In following, thermodynamic parameters for the products including energetic levels, HOMO and LUMO parameters, chemical hardness, electrophilicity and chemical potential for this structures were calculated by using the density functional theory in method and B3LYP/6-311G(d,p) level of theory.
Doi 10.13005/ojc/280149
Is Certified Translation No
Dupe Override No
Comments Scopus URL: https://www.scopus.com/inward/record.uri?eid=2-s2.0-84861856021&doi=10.13005%2fojc%2f280149&partnerID=40&md5=f0020d8a5647c3b99a64ff4119433418
Is Public Yes
Language Text English
Keyword DFT; Electrophilicity; Mannich reaction; Synthesis