Preparation of ammonium diuranate particles by external gelation process of uranium in INET

Zhou Xiangwen; Ma Jingtao; Hao Shaochang; Zhao Xingyu; Wang Yang; Deng Changsheng; Liang Tongxiang; Guo Wenli; Tang Yaping; Tang Chunhe

HERO ID

1611583

Reference Type

Journal Article

Year

2012

HERO ID 1611583
In Press No
Year 2012
Title Preparation of ammonium diuranate particles by external gelation process of uranium in INET
Authors Zhou Xiangwen; Ma Jingtao; Hao Shaochang; Zhao Xingyu; Wang Yang; Deng Changsheng; Liang Tongxiang; Guo Wenli; Tang Yaping; Tang Chunhe
Journal Nuclear Engineering and Design
Volume 250
Page Numbers 192-196
Abstract In order to satisfy the mass spherical fuel elements (SFE) requirements for the High Temperature gas-cooled Reactor (HTR)-Pebble bed Module (HTR-PM), a modified and optimized fabrication of dense uranium dioxide (UO2) kernel via an acid-deficiency uranium nitrate (ADUN) solution was researched and developed in the institute of nuclear and new energy technology (INET). In this study, external gelation process of uranium (EGU) based on the total gelation of uranium (TGU) in the period of 10 MW HTR (HTR-10) was used to prepare the ammonium diuranate (ADU) compound particles, an intermediate for UO2 kernel. The scale of batch production was improved from 500g U/batch at that time to current 3 kg U/batch. Improvements in many aspects such as large scale preparation of ADUN, multiple-nozzle casting system and new aging, washing and drying (AWD) system without isopropanol were also presented. Under strict controls and measures. ADU particles with good sphericity and uniform diameter were acquired to ensure the subsequent preparation of dense UO2 kernels for HTR-PM. (C) 2012 Elsevier B.V. All rights reserved.
Doi 10.1016/j.nucengdes.2012.06.001
Wosid WOS:000308266500021
Is Certified Translation No
Dupe Override No
Comments Source: Web of Science WOS:000308266500021
Is Public Yes