Ternary blend all-polymer solar cells: enhanced performance and evidence of parallel-like bulk heterojunction mechanism

Hwang, Y; Courtright, BAE; Jenekhe, SA

HERO ID

3125588

Reference Type

Journal Article

Year

2015

Language

English

HERO ID 3125588
In Press No
Year 2015
Title Ternary blend all-polymer solar cells: enhanced performance and evidence of parallel-like bulk heterojunction mechanism
Authors Hwang, Y; Courtright, BAE; Jenekhe, SA
Volume 5
Issue 2
Page Numbers 229-234
Abstract All-polymer solar cells composed of binary blends of donor poly[4,8-bis(5-(2-ethylhexyl)thiophen-2-yl)benzo[1,2-b;4,5-b']dithiophene-2,6-diyl-alt-(4-(2-ethylhexanoyl)-thieno[3,4-b]thiophene-)-2-6-diyl)] (PBDTTT-CT), and acceptor polymers naphthalene diimide-selenophene copolymer (PNDIS-HD) and perylene diimide-selenophene copolymer (PPDIS) had power conversion efficiencies (PCEs) of 1.3 and 2.1%, respectively. Ternary blend solar cells composed of [PBDTTT-CT][PNDIS-HD](1-x)[PPDIS](x) at 75 wt% PPDIS had a PCE of 3.2%, which is about a 50%-140% enhancement compared with the binary blend devices. Equality of the ternary blend short-circuit current to the sum of those of the binary blend devices, among other results, provided evidence of a parallel-like bulk heterojunction mechanism in the ternary blend solar cells. These results provide the first example of enhanced performance in ternary blend all-polymer solar cells.
Doi 10.1557/mrc.2015.36
Wosid WOS:000358147300011
Url https://www.scopus.com/inward/record.uri?eid=2-s2.0-84946473980&doi=10.1557%2fmrc.2015.36&partnerID=40&md5=b529481e8f95ac79831da1954e3b11a3
Is Certified Translation No
Dupe Override No
Comments Journal:MRS COMMUNICATIONS 2159-6859
Is Public Yes
Language Text English