Analysis and characterization of iron pyrite nanocrystals and nanocrystalline thin films derived from bromide anion synthesis

Bhandari, KP; Roland, PJ; Kinner, T; Cao, Y; Choi, H; Jeong, S; Ellingson, RJ

HERO ID

4683976

Reference Type

Journal Article

Year

2015

HERO ID 4683976
In Press No
Year 2015
Title Analysis and characterization of iron pyrite nanocrystals and nanocrystalline thin films derived from bromide anion synthesis
Authors Bhandari, KP; Roland, PJ; Kinner, T; Cao, Y; Choi, H; Jeong, S; Ellingson, RJ
Volume 3
Issue 13
Page Numbers 6853-6861
Abstract We use a solution-based hot injection method to synthesize stable, phase pure and highly crystalline cubic iron pyrite (FeS2) nanocrystals, with size varying from similar to 70 to 150 nm. We use iron(II) bromide as an iron precursor, elemental sulfur as the sulfur source, trioctylphosphine oxide (TOPO) and 1,2-hexanediol as capping ligands, and oleylamine (OLA) as a non-coordinating solvent during the synthesis. We report on the influence of hydrazine treatment, and of thermal sintering, on the morphological, electronic, optical, and surface chemical properties of FeS2 films. Four point probe and Hall measurements indicate that these iron pyrite films are highly conductive. Although they are unsuitable as an effective photovoltaic light-absorbing layer, they offer clear potential as a conducting contact layer in photovoltaic and other optoelectronic devices.
Doi 10.1039/c4ta06320a
Wosid WOS:000351552300020
Is Certified Translation No
Dupe Override No
Comments Journal:JOURNAL OF MATERIALS CHEMISTRY A 2050-7488
Is Public Yes