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7225363 
Journal Article 
Impact of alternating current electric field poling on piezoelectric and dielectric properties of Pb(In1/2Nb1/2)O-3-Pb(Mg1/3Nb2/3)O-3-PbTiO3 ferroelectric crystals 
Liu, J; Qiu, C; Qiao, L; Song, K; Guo, H; Xu, Z; Li, Fei; , 
2020 
No 
Journal of Applied Physics
ISSN: 0021-8979
EISSN: 1089-7550 
AMER INST PHYSICS 
MELVILLE 
128 
9 
English 
WOS:000568568300001 
Compared with the state-of-the-art Pb(Zr,Ti)O-3 ceramics, relaxor-PbTiO3 (PT) based ferroelectric single crystals possess much higher piezoelectricity, thus receiving considerable attention from the ferroelectric community. Recently, it was found that the alternating current electric field poling (AC-poling) could further improve the piezoelectricity of [001]-poled rhombohedral (R) relaxor-PT single crystals. In this work, we investigated the domain structures and electromechanical properties of alternating current electric field poled (AC-poled) relaxor ferroelectric Pb(In1/2Nb1/2)O-3-Pb(Mg1/3Nb2/3)O-3-PbTiO3 (PIN-PMN-PT) crystals with different orientations and phase structures, including [001]-oriented R PIN-PMN-PT (23/47/30), [011]-oriented R PIN-PMN-PT (23/47/30), and [001]-oriented monoclinic (M-C) PIN-PMN-PT (22/44/34) single crystals. We found that the piezoelectric coefficient (d(33)), free dielectric permittivity ((T)(33)/(0)), and clamped dielectric permittivity ((S)(33)/(0)) for AC-poled [001]-oriented R PIN-PMN-PT (23/47/30) crystals were improved by 24.4%, 22.6%, and 8.5%, respectively, when compared with the direct current electric field poled (DC-poled) counterparts. This phenomenon is attributed to the increase of domain size according to the observations from polarized light microscopy. Nevertheless, for [011]-poled R PIN-PMN-PT and [001]-poled M-C PIN-PMN-PT crystals, the dielectric permittivities and piezoelectric coefficients were decreased a bit by AC-poling, being attributed to the depolarization phenomenon caused by the AC electric field. This work demonstrates that impacts of AC-poling on the properties of ferroelectrics are highly related to the orientation and phase of ferroelectric crystals. 
JOURNAL OF APPLIED PHYSICS