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Citation
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HERO ID
8493540
Reference Type
Journal Article
Title
Neutron scattering experiments and computer simulation studies of a polymer electrolyte
Author(s)
Carlsson, P
Year
1999
Publisher
Chalmers Tekniska Hogskola
Location
Goteborg, Sweden
Issue
1532
Page Numbers
1-75
Language
English
Abstract
The microscopic structure and dynamics of a solvent free polymer electrolyte, polypropylene oxide complexed with LiClO4, is presented. The structure was studied using neutron and X-ray diffraction experiments combined with reverse Monte Carlo and Molecular Dynamics simulations. Results show that for low salt concentrations, the inter-chain distance is constant, indicating a large excess volume between the chains which can host the salt. Furthermore, a significant polymer-anion and inter-anionic correlations were found indicating an inhomogeneous distribution of the salt on intermediate length scales.
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