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HERO ID
8716399
Reference Type
Journal Article
Title
Three/Four/Five-Component Diastereoselective Cyclization of Fischer Carbene Complexes, Lithium Enolates, and Allylmagnesium Bromide
Author(s)
Barluenga, J; Pérez-Sánchez, I; Rubio, E; Flórez, J
Year
2003
Is Peer Reviewed?
Yes
Journal
Angewandte Chemie (International Edition)
ISSN:
1433-7851
EISSN:
1521-3773
Volume
42
Issue
47
Page Numbers
5860-5863
Language
English
DOI
10.1002/anie.200352489
Abstract
From three simple starting materials, the diastereoselective synthesis of pentasubstituted cyclopentanols or tetrasubstituted cyclohexane-1,4-diols can be controlled by the appropriate choice of lithium enolate (see scheme). The overall one-pot transformation leads to the formation of up to five new C-C bonds and up to four contiguous stereogenic centers.
Keywords
Carbenes; Chromium; Cyclization; Enolates multicomponent reactions
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